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Yang, Yang; Wang, Yiping; Rousochatzakis, Ioannis; Ruiz, Alejandro; Analytis, James G.; Burch, Kenneth S.; Perkins, Natalia B. (, Physical Review B)
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Ruiz, Alejandro; Gunn, Brandon; Lu, Yi; Sasmal, Kalyan; Moir, Camilla M.; Basak, Rourav; Huang, Hai; Lee, Jun-Sik; Rodolakis, Fanny; Boyle, Timothy J.; et al (, Nature Communications)Abstract The shape of 3d-orbitals often governs the electronic and magnetic properties of correlated transition metal oxides. In the superconducting cuprates, the planar confinement of the$${d}_{{x}^{2}-{y}^{2}}$$ orbital dictates the two-dimensional nature of the unconventional superconductivity and a competing charge order. Achieving orbital-specific control of the electronic structure to allow coupling pathways across adjacent planes would enable direct assessment of the role of dimensionality in the intertwined orders. Using CuL3and PrM5resonant x-ray scattering and first-principles calculations, we report a highly correlated three-dimensional charge order in Pr-substituted YBa2Cu3O7, where the Prf-electrons create a direct orbital bridge between CuO2planes. With this we demonstrate that interplanar orbital engineering can be used to surgically control electronic phases in correlated oxides and other layered materials.more » « less
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Michielsen, Koen; Rodríguez‐Ruiz, Alejandro; Reiser, Ingrid; Nagy, James G.; Sechopoulos, Ioannis (, Medical Physics)null (Ed.)
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Ruiz, Alejandro; Nagarajan, Vikram; Vranas, Mayia; Lopez, Gilbert; McCandless, Gregory T.; Kimchi, Itamar; Chan, Julia Y.; Breznay, Nicholas P.; Frañó, Alex; Frandsen, Benjamin A.; et al (, Physical Review B)
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Kang, Mingu; Pelliciari, Jonathan; Frano, Alex; Breznay, Nicholas; Schierle, Enrico; Weschke, Eugen; Sutarto, Ronny; He, Feizhou; Shafer, Padraic; Arenholz, Elke; et al (, Nature Physics)
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